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I agree the rear of the hood needs to come down. The side to side gap doesn't look too bad from here.
This is the "tell": the fenders have no adjustability at the rad support. They bolt up solid (with no shims or anything). That establishes the side to side gap at the front of the hood. Take that gap and that's what you want to run rearward (so that it is uniform all the way back).
The top of the fenders attach to the cab with one vertical bolt and one horizontal bolt. There may be shims in there; if there are shims present you can remove them and bring the fenders in if you want. Both the horizontal bolt and the vertical bolt will need to be loosened in order to move the fender. If there are no shims then they are as far inboard as they will go and you can't do anything without some serious metalwork.
If that makes the leading edge of the door stick you then those will need to move inboard, too, by moving the door on the hinges.
You might decide after all this that the hood gap looks pretty good